Generalized Transition Moment and Oscillator Strength for Optimal Control of Excited States Using Near-Field Light.
Abstract
The near field is a highly localized light field that is present in the vicinity of materials. It holds considerable potential for manipulating molecular excitation through the design of nanostructures. To that end, a simple yet applicable computational method is required. This letter presents an optimization strategy to achieve targeted electronic excitation in molecules using near-field light. The generalized transition moment and oscillator strength based on the multipolar Hamiltonian can…
Read the original article on The Journal of Physical Chemistry Letters
Article Information:
Takeshi Iwasa
Generalized Transition Moment and Oscillator Strength for Optimal Control of Excited States Using Near-Field Light
The Journal of Physical Chemistry Letters, 26 April 2024.
DOI: 10.1021/acs.jpclett.4c00609
